Non-Directed, Pd-Catalyzed C-H Amination of Simple Arenes
Abstract
We describe the first Pd catalyzed method for the
one-step C H amination of simple arenes. The activity of the
catalysts is highly dependent on the Pd:ligand ratio and the
identity of the used ligands. Turnover numbers up to 12 can be
achieved.
one-step C H amination of simple arenes. The activity of the
catalysts is highly dependent on the Pd:ligand ratio and the
identity of the used ligands. Turnover numbers up to 12 can be
achieved.
Keywords
sp2 C-H amination, non-directed C-H activation, palladium/pyridine catalysts, oxidant.
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